Vacancy-type defects and electronic structure of perovskite-oxide SrTiO 3 from positron annihilation

A. S. Hamid, A. Uedono, T. Chikyow, K. Uwe, K. Mochizuki, S. Kawaminami

研究成果: Article査読

12 被引用数 (Scopus)

抄録

The vacancy-type defects in Nb-doped SrTiO 3 and in undoped SrTiO 3, annealed in H 2 flow, were investigated by means of positron lifetime and 2D angular correlation of annihilation radiation (ACAR) experiments. The calculations of the lifetime of positron were performed by using atomic superposition (AT-SUP) method. The results showed that positrons annihilate from a free state in the Nb-doped SrTiO 3. The trapping centers in the annealed sample were found to be oxygen vacancies V o associated with relaxation of the surrounding ions. Moreover, the momentum distributions of the samples studied were correlated to the variation of their electronic structure. It was proposed from the drastic change in the momentum distribution upon introduction of V o, that 2D-ACAR technique is a sensitive tool for acquiring information on the electronic and bond structure of the perovskite-oxides.

本文言語English
ページ(範囲)300-305
ページ数6
ジャーナルPhysica Status Solidi (A) Applications and Materials Science
203
2
DOI
出版ステータスPublished - 2006 2 1
外部発表はい

ASJC Scopus subject areas

  • 電子材料、光学材料、および磁性材料
  • 凝縮系物理学
  • 表面および界面
  • 表面、皮膜および薄膜
  • 電子工学および電気工学
  • 材料化学

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