Ultrafast extreme ultraviolet induced isomerization of acetylene cations

Y. H. Jiang; A. Rudenko; O. Herrwerth; L. Foucar; M. Kurka; K. U. Kühnel; M. Lezius; M. F. Kling; J. Van Tilborg; A. Belkacem; K. Ueda; S. Düsterer; R. Treusch; C. D. Schröter; R. Moshammer; J. Ullrich

doi:10.1103/PhysRevLett.105.263002

Ultrafast extreme ultraviolet induced isomerization of acetylene cations

Y. H. Jiang, A. Rudenko, O. Herrwerth, L. Foucar, M. Kurka, K. U. Kühnel, M. Lezius, M. F. Kling, J. Van Tilborg, A. Belkacem, K. Ueda, S. Düsterer, R. Treusch, C. D. Schröter, R. Moshammer, J. Ullrich

多元物質科学研究所・計測研究部門

研究成果: Article › 査読

152 被引用数 (Scopus)

抄録

Ultrafast isomerization of acetylene cations ([HC=CH]⊃+) in the low-lying excited AΣg+2 state, populated by the absorption of extreme ultraviolet (XUV) photons (38 eV), has been observed at the Free Electron Laser in Hamburg, (FLASH). Recording coincident fragments C⊃++CH2+ as a function of time between XUV-pump and -probe pulses, generated by a split-mirror device, we find an isomerization time of 52±15fs in a kinetic energy release (KER) window of 5.8<KER<8eV, providing clear evidence for the existence of a fast, nonradiative decay channel.

本文言語	English
論文番号	263002
ジャーナル	Physical review letters
巻	105
号	26
DOI	https://doi.org/10.1103/PhysRevLett.105.263002
出版ステータス	Published - 2010 12 22

ASJC Scopus subject areas

物理学および天文学（全般）

文献へのアクセス

10.1103/PhysRevLett.105.263002

他のファイルとリンク

引用スタイル

Jiang, Y. H., Rudenko, A., Herrwerth, O., Foucar, L., Kurka, M., Kühnel, K. U., Lezius, M., Kling, M. F., Van Tilborg, J., Belkacem, A., Ueda, K., Düsterer, S., Treusch, R., Schröter, C. D., Moshammer, R., & Ullrich, J. (2010). Ultrafast extreme ultraviolet induced isomerization of acetylene cations. Physical review letters, 105(26), [263002]. https://doi.org/10.1103/PhysRevLett.105.263002

Ultrafast extreme ultraviolet induced isomerization of acetylene cations. / Jiang, Y. H.; Rudenko, A.; Herrwerth, O.; Foucar, L.; Kurka, M.; Kühnel, K. U.; Lezius, M.; Kling, M. F.; Van Tilborg, J.; Belkacem, A.; Ueda, K.; Düsterer, S.; Treusch, R.; Schröter, C. D.; Moshammer, R.; Ullrich, J.

In: Physical review letters, Vol. 105, No. 26, 263002, 22.12.2010.

研究成果: Article › 査読

Jiang, YH, Rudenko, A, Herrwerth, O, Foucar, L, Kurka, M, Kühnel, KU, Lezius, M, Kling, MF, Van Tilborg, J, Belkacem, A, Ueda, K, Düsterer, S, Treusch, R, Schröter, CD, Moshammer, R & Ullrich, J 2010, 'Ultrafast extreme ultraviolet induced isomerization of acetylene cations', Physical review letters, vol. 105, no. 26, 263002. https://doi.org/10.1103/PhysRevLett.105.263002

@article{9e15dae754d24f6ea8840792863c62fd,

title = "Ultrafast extreme ultraviolet induced isomerization of acetylene cations",

abstract = "Ultrafast isomerization of acetylene cations ([HC=CH]⊃+) in the low-lying excited AΣg+2 state, populated by the absorption of extreme ultraviolet (XUV) photons (38 eV), has been observed at the Free Electron Laser in Hamburg, (FLASH). Recording coincident fragments C⊃++CH2+ as a function of time between XUV-pump and -probe pulses, generated by a split-mirror device, we find an isomerization time of 52±15fs in a kinetic energy release (KER) window of 5.8<KER<8eV, providing clear evidence for the existence of a fast, nonradiative decay channel.",

author = "Jiang, {Y. H.} and A. Rudenko and O. Herrwerth and L. Foucar and M. Kurka and K{\"u}hnel, {K. U.} and M. Lezius and Kling, {M. F.} and {Van Tilborg}, J. and A. Belkacem and K. Ueda and S. D{\"u}sterer and R. Treusch and Schr{\"o}ter, {C. D.} and R. Moshammer and J. Ullrich",

year = "2010",

month = dec,

day = "22",

doi = "10.1103/PhysRevLett.105.263002",

language = "English",

volume = "105",

journal = "Physical Review Letters",

issn = "0031-9007",

publisher = "American Physical Society",

number = "26",

}

TY - JOUR

T1 - Ultrafast extreme ultraviolet induced isomerization of acetylene cations

AU - Jiang, Y. H.

AU - Rudenko, A.

AU - Herrwerth, O.

AU - Foucar, L.

AU - Kurka, M.

AU - Kühnel, K. U.

AU - Lezius, M.

AU - Kling, M. F.

AU - Van Tilborg, J.

AU - Belkacem, A.

AU - Ueda, K.

AU - Düsterer, S.

AU - Treusch, R.

AU - Schröter, C. D.

AU - Moshammer, R.

AU - Ullrich, J.

PY - 2010/12/22

Y1 - 2010/12/22

N2 - Ultrafast isomerization of acetylene cations ([HC=CH]⊃+) in the low-lying excited AΣg+2 state, populated by the absorption of extreme ultraviolet (XUV) photons (38 eV), has been observed at the Free Electron Laser in Hamburg, (FLASH). Recording coincident fragments C⊃++CH2+ as a function of time between XUV-pump and -probe pulses, generated by a split-mirror device, we find an isomerization time of 52±15fs in a kinetic energy release (KER) window of 5.8<KER<8eV, providing clear evidence for the existence of a fast, nonradiative decay channel.

AB - Ultrafast isomerization of acetylene cations ([HC=CH]⊃+) in the low-lying excited AΣg+2 state, populated by the absorption of extreme ultraviolet (XUV) photons (38 eV), has been observed at the Free Electron Laser in Hamburg, (FLASH). Recording coincident fragments C⊃++CH2+ as a function of time between XUV-pump and -probe pulses, generated by a split-mirror device, we find an isomerization time of 52±15fs in a kinetic energy release (KER) window of 5.8<KER<8eV, providing clear evidence for the existence of a fast, nonradiative decay channel.

UR - http://www.scopus.com/inward/record.url?scp=78650483371&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=78650483371&partnerID=8YFLogxK

U2 - 10.1103/PhysRevLett.105.263002

DO - 10.1103/PhysRevLett.105.263002

M3 - Article

AN - SCOPUS:78650483371

VL - 105

JO - Physical Review Letters

JF - Physical Review Letters

SN - 0031-9007

IS - 26

M1 - 263002

ER -

Ultrafast extreme ultraviolet induced isomerization of acetylene cations

抄録

ASJC Scopus subject areas

文献へのアクセス

他のファイルとリンク

フィンガープリント

引用スタイル