Two-dome structure in electron-doped iron arsenide superconductors

Soshi Iimura, Satoru Matuishi, Hikaru Sato, Taku Hanna, Yoshinori Muraba, Sung Wng Kim, Jung Eun Kim, Masaki Takata, Hideo Hosono

研究成果: Article査読

149 被引用数 (Scopus)


Iron arsenide superconductors based on the material LaFeAsO 1-x F x are characterized by a two-dimensional Fermi surface (FS) consisting of hole and electron pockets yielding structural and antiferromagnetic transitions at x=0. Electron doping by substituting O 2- with F - suppresses these transitions and gives rise to superconductivity with a maximum T c of 26 K at x=0.1. However, the over-doped region cannot be accessed due to the poor solubility of F - above x=0.2. Here we overcome this problem by doping LaFeAsO with hydrogen. We report the phase diagram of LaFeAsO 1-x H x (x<0.53) and, in addition to the conventional superconducting dome seen in LaFeAsO 1-x F x, we find a second dome in the range 0.21<x<0.53, with a maximum T c of 36 K at x=0.3. Density functional theory calculations reveal that the three Fe 3d bands (xy, yz and zx) become degenerate at x=0.36, whereas the FS nesting is weakened monotonically with x. These results imply that the band degeneracy has an important role to induce high T c.

ジャーナルNature communications
出版ステータスPublished - 2012

ASJC Scopus subject areas

  • 化学 (全般)
  • 生化学、遺伝学、分子生物学(全般)
  • 物理学および天文学(全般)


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