95Tc and96Tc production by (γ, xn) reactions

T. Sekine, K. Yoshihara, J. Sáfár, L. Lakosi, A. Veres

研究成果: Article査読

3 被引用数 (Scopus)

抄録

The99Tc (γ, 3n)96Tc and99Tc (γ, 4n)95Tc reactions were studied by irradiation of target99Tc with bremsstrahlung from the linear electron accelerator of Tohoku University, up to 50 MeV γ-energy. The resulting96Tc (4.3 d) and95Tc (20 h) activities were determined by γ-spectrometry. The γ-flux was monitored by the99Tc (γ, γ′)99mTc reaction. Metallic copper and gold foils were used as additional flux monitors in front of and behind the samples. Their measured radioactivity was utilized for normalizing bremsstrahlung flux calculations, in order to determine reaction cross sections. Cross sections were also determined theoretically, performing calculations in the framework of a neutron cascade evaporation model. Above the (γ, 3n) and (γ, 4n) threshold energies the neutron emission channel was supposed to be the only open channel for deexcitation following photoabsorption. The preeguilibrium contribution was considered negligible. The experimental results obtained for the integrated cross section at 30 and 50 MeV fit reasonably well the calculated curves.

本文言語English
ページ(範囲)165-174
ページ数10
ジャーナルJournal of Radioanalytical and Nuclear Chemistry Letters
186
2
DOI
出版ステータスPublished - 1994 1月 1

ASJC Scopus subject areas

  • 分析化学
  • 原子力エネルギーおよび原子力工学
  • 放射線学、核医学およびイメージング
  • 汚染
  • 分光学
  • 公衆衛生学、環境および労働衛生
  • 健康、毒物学および変異誘発

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