Quasielastic light scattering from rutile

A. Koreeda, M. Yoshizawa, S. Saikan

研究成果: Article査読

12 被引用数 (Scopus)

抄録

Quasielastic light scattering consisting of two components has been observed in single crystals of rutile (Formula presented) The broad component with a linewidth of 330 GHz at 297 K becomes narrower with decreasing temperature. In contrast, the narrow component, which has a linewidth of 1.1 GHz at 297 K, broadens as the temperature decreases. We present a unified explanation for both components, which is based on two-phonon difference Raman scattering. For the narrow component, it will be shown that two-phonon difference processes from a single acoustic phonon branch explain the temperature dependence of the intensity and the wave vector dependence of the linewidth at low temperatures. The conventional explanation in terms of entropy-fluctuation scattering is also attempted for temperatures above 200 K where phonon collisions occur more frequently than at lower temperatures and the phonon system may be considered hydrodynamically. For the broad component, two-phonon difference scattering from different phonon branches will be shown to provide a good explanation for the temperature dependent intensity. Furthermore, temperature dependence of the linewidth and its insensitivity to changes in scattering wave vector are also explained with this model.

本文言語English
ページ(範囲)12730-12736
ページ数7
ジャーナルPhysical Review B - Condensed Matter and Materials Physics
60
18
DOI
出版ステータスPublished - 1999

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

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