TY - JOUR
T1 - Process assessments for low-temperature methane reforming using oxygen carrier metal oxide nanoparticles
AU - Yoko, Akira
AU - Fukushima, Yasuhiro
AU - Shimizu, Tadaaki
AU - Kikuchi, Yasunori
AU - Shimizu, Teruyuki
AU - Guzman-Urbina, Alexander
AU - Ouchi, Kakeru
AU - Hirai, Haruka
AU - Seong, Gimyeong
AU - Tomai, Takaaki
AU - Adschiri, Tadafumi
N1 - Funding Information:
This work was supported by the Japan Science and Technology Agency (JST) [MIRAI; Grant Number JPMJMI17E4 and CREST ; Grant Number JPMJCR16P3 ], the New Energy and Industrial Technology Development Organization of Japan (NEDO), JSPS KAKENHI [ 16H06367 and 16H06126 ], and World Premier International Research Center Initiative (WPI), MEXT , Japan. The Presidential Endowed Chair for the “Platinum Society” in the University of Tokyo is supported by the KAITEKI Institute Incorporated, Mitsui Fudosan Corporation, Shin-Etsu Chemical Co., ORIX Corporation, Sekisui House, Ltd., and the East Japan Railway Company.
Publisher Copyright:
© 2019 Elsevier B.V.
PY - 2019/8
Y1 - 2019/8
N2 - The utilization of low-temperature waste heat in the endothermic hydrocarbon reforming reaction can improve the energy efficiency of the chemical product synthesis system. In this study, process assessments are conducted, and potential technologies to realize the reforming process using low-temperature waste heat are discussed. Based on the assessment and process design, a low-temperature methane reforming process using circulating fluidized beds is proposed. An investigation into the use of metal oxide nanoparticles fabricated by the supercritical method as an oxygen carrier serves as a partial proof-of-concept for the low-temperature reforming process. The requirements for the oxygen carrier in the process are calculated based on a target for the amount of methane reformed in the methanol production plant.
AB - The utilization of low-temperature waste heat in the endothermic hydrocarbon reforming reaction can improve the energy efficiency of the chemical product synthesis system. In this study, process assessments are conducted, and potential technologies to realize the reforming process using low-temperature waste heat are discussed. Based on the assessment and process design, a low-temperature methane reforming process using circulating fluidized beds is proposed. An investigation into the use of metal oxide nanoparticles fabricated by the supercritical method as an oxygen carrier serves as a partial proof-of-concept for the low-temperature reforming process. The requirements for the oxygen carrier in the process are calculated based on a target for the amount of methane reformed in the methanol production plant.
KW - Chemical looping
KW - Low-temperature methane reforming
KW - Methanol production
KW - Oxygen carrier
KW - Process assessment
KW - Waste heat
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U2 - 10.1016/j.cep.2019.107531
DO - 10.1016/j.cep.2019.107531
M3 - Article
AN - SCOPUS:85066437050
VL - 142
JO - Chemical Engineering and Processing: Process Intensification
JF - Chemical Engineering and Processing: Process Intensification
SN - 0255-2701
M1 - 107531
ER -