Post-growth annealing effects on charge and spin excitations in Nd2-xCexCuO4

Kenji Ishii, Shun Asano, Masumi Ashida, Masaki Fujita, Biqiong Yu, Martin Greven, Jun Okamoto, Di Jing Huang, Jun'Ichiro Mizuki

研究成果: Article査読

4 被引用数 (Scopus)


We report a Cu K- and L3-edge resonant inelastic x-ray scattering study of charge and spin excitations of bulk Nd2-xCexCuO4, with a focus on post-growth annealing effects. For the parent compound Nd2CuO4 (x=0), a clear charge-transfer gap is observed in the as-grown state, whereas the charge excitation spectra indicate that electrons are doped in the annealed state. This is consistent with the observation that annealed thin-film and polycrystalline samples of RE2CuO4 (RE=rare earth) can become metallic and superconducting at sufficiently high electron concentrations without Ce doping. For x=0.16, a Ce concentration for which it is known that oxygen reduction destroys long-range antiferromagnetic order and induces superconductivity, we find that the high-energy spin excitations of non-superconducting as-grown and superconducting annealed crystals are nearly identical. This finding is in stark contrast to the significant changes in the low-energy spin excitations previously observed via neutron scattering.

ジャーナルPhysical Review Materials
出版ステータスPublished - 2021 2月

ASJC Scopus subject areas

  • 材料科学(全般)
  • 物理学および天文学(その他)


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