Optimal control approaches for aligning/orienting asymmetric top molecules

Yukiyoshi Ohtsuki, Masataka Yoshida, Yuta Arakawa

研究成果: Chapter

抄録

We explain optimal control approaches with the aim of three-dimensional (3D) alignment/orientation of asymmetric molecules by using a combination of dipole and lowest-order-induced dipole interactions, the former of which mixes the rotational states with different parity. The present method enables the numerical design of an optimal temporal structure for the laser pulse including its time-dependent polarization on the basis of the molecular Hamiltonian together with the optimization algorithm. After explaining the theoretical framework, numerical details are examined through a case study of one-dimensional (1D) alignment control that is applied to SO2.

本文言語English
ホスト出版物のタイトルSpringer Series in Chemical Physics
出版社Springer New York LLC
ページ65-79
ページ数15
DOI
出版ステータスPublished - 2018 1 1

出版物シリーズ

名前Springer Series in Chemical Physics
118
ISSN(印刷版)0172-6218

ASJC Scopus subject areas

  • Physical and Theoretical Chemistry

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