Multipole orders and fluctuations in strongly correlated electron systems

Yoshio Kuramoto, Hiroaki Kusunose, Annamária Kiss

研究成果: Article査読

182 被引用数 (Scopus)

抄録

In this paper we review experimental and theoretical results on higher electronic multipoles in solids with strong correlations. Recent experiments and their theoretical interpretation have confirmed the ordering of octupoles and even higher multipoles in rare-earth and actinide compounds withf electrons. The concept of multipoles is critically examined in point groups where spherical tensors of different ranks mix. Using a phenomenological approach, we demonstrate how linear and nonlinear couplings of different multipoles lead to rich phase diagrams and anomalies in physical observables. As actual representative systems, we first consider CexLa 1-xB 6, for which resonant X-ray scattering probed the octupole order for the first time, and NpO 2, where quadrupoles induced by the octupole order have been observed. We then consider a class of compounds called skutterudites as the most convenient system for systematic study. Particular emphasis is placed on the ordering of scalar components from fourth-rank tensors (hexadecapoles) and sixth-rank tensors (hexacontatetrapoles). A comparison of a skutterudite PrFe 4P1 2and URu 2Si 2 is made, where much fewer carriers remain in the ordered states than in the disordered phase. The even number (two) off electrons per site in Pr 3+ or U 4+ makes the system free from the Kramers degeneracy, in contrast to standard models for Mott transitions. Hence, it is pointed out that multipole orders, particularly the scalar order, should provide a new route for studying the dichotomy between the itinerant and localized behaviors of electrons.

本文言語English
論文番号072001
ジャーナルjournal of the physical society of japan
78
7
DOI
出版ステータスPublished - 2009 7 1

ASJC Scopus subject areas

  • 物理学および天文学(全般)

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