TY - JOUR
T1 - Continuum limit of the vibrational properties of amorphous solids
AU - Mizuno, Hideyuki
AU - Shiba, Hayato
AU - Ikeda, Atsushi
N1 - Funding Information:
ACKNOWLEDGMENTS. We thank H. Ikeda, Y. Jin, L. E. Silbert, P. Charbonneau, F. Zamponi, L. Berthier, E. Lerner, E. Bouchbinder, and K. Miyazaki for useful discussions and suggestions. This work was supported by Japan Society for the Promotion of Science Grant-in-Aid for Young Scientists B 17K14369, Grant-in-Aid for Young Scientists A 17H04853, and Grant-in-Aid for Scientific Research B 16H04034. The numerical calculations were partly performed on SGI Altix ICE XA at the Institute for Solid State Physics, The University of Tokyo.
Publisher Copyright:
© 2017, National Academy of Sciences. All rights reserved.
PY - 2017/11/14
Y1 - 2017/11/14
N2 - The low-frequency vibrational and low-temperature thermal properties of amorphous solids are markedly different from those of crystalline solids. This situation is counterintuitive because all solid materials are expected to behave as a homogeneous elastic body in the continuum limit, in which vibrational modes are phonons that follow the Debye law. A number of phenomenological explanations for this situation have been proposed, which assume elastic heterogeneities, soft localized vibrations, and so on. Microscopic mean-field theories have recently been developed to predict the universal non-Debye scaling law. Considering these theoretical arguments, it is absolutely necessary to directly observe the nature of the low-frequency vibrations of amorphous solids and determine the laws that such vibrations obey. Herein, we perform an extremely large-scale vibrational mode analysis of a model amorphous solid. We find that the scaling law predicted by the mean-field theory is violated at low frequency, and in the continuum limit, the vibrational modes converge to a mixture of phonon modes that follow the Debye law and soft localized modes that follow another universal non-Debye scaling law.
AB - The low-frequency vibrational and low-temperature thermal properties of amorphous solids are markedly different from those of crystalline solids. This situation is counterintuitive because all solid materials are expected to behave as a homogeneous elastic body in the continuum limit, in which vibrational modes are phonons that follow the Debye law. A number of phenomenological explanations for this situation have been proposed, which assume elastic heterogeneities, soft localized vibrations, and so on. Microscopic mean-field theories have recently been developed to predict the universal non-Debye scaling law. Considering these theoretical arguments, it is absolutely necessary to directly observe the nature of the low-frequency vibrations of amorphous solids and determine the laws that such vibrations obey. Herein, we perform an extremely large-scale vibrational mode analysis of a model amorphous solid. We find that the scaling law predicted by the mean-field theory is violated at low frequency, and in the continuum limit, the vibrational modes converge to a mixture of phonon modes that follow the Debye law and soft localized modes that follow another universal non-Debye scaling law.
KW - Amorphous solids
KW - Continuum limit
KW - Non-Debye law
KW - Phonons
KW - Soft localized modes
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U2 - 10.1073/pnas.1709015114
DO - 10.1073/pnas.1709015114
M3 - Article
C2 - 29087941
AN - SCOPUS:85033687860
VL - 114
SP - E9767-E9774
JO - Proceedings of the National Academy of Sciences of the United States of America
JF - Proceedings of the National Academy of Sciences of the United States of America
SN - 0027-8424
IS - 46
ER -