Coherent transfer via environment-induced vibronic resonance

Hiroyuki Tamura

    研究成果: Article査読

    9 被引用数 (Scopus)

    抄録

    We systematically analyze vibronic dynamics considering a high-frequency system mode and low-frequency environmental modes by using quantum dynamics calculations. We demonstrate how the vibronic resonance and environment dynamics induce a coherent transfer between coupled electronic states with a potential energy bias. The concerted dynamics of the low-frequency modes modulates the potential crossing, thereby inducing a coherent population transfer when the resonance condition is matched. This feature would underlie transfer phenomena in certain realistic systems.

    本文言語English
    論文番号214705
    ジャーナルJournal of Chemical Physics
    130
    21
    DOI
    出版ステータスPublished - 2009

    ASJC Scopus subject areas

    • Physics and Astronomy(all)
    • Physical and Theoretical Chemistry

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