Application of stochastic Liouville-von Neumann equation to electronic energy transfer in FMO complex

Hajime Imai, Yukiyoshi Ohtsuki, Hirohiko Kono

研究成果: Article査読

12 被引用数 (Scopus)

抄録

A stochastic Liouville-von Neumann approach to solving a spin-boson model is applied to electronic energy transfer in Fenna-Matthews-Olson (FMO) complexes as a case study of the dynamics in biological systems. We modify a noise generation method to treat an experimentally obtained highly structured spectral density. By considering the population dynamics in a two-site system with a model structured spectral density, we numerically observe two kinds of coherent motions associated with inter-site coupling and system-bath coupling, the latter of which is mainly attributed to the peak structure of the spectral density.

本文言語English
ページ(範囲)134-141
ページ数8
ジャーナルChemical Physics
446
DOI
出版ステータスPublished - 2015 8月 9

ASJC Scopus subject areas

  • 物理学および天文学(全般)
  • 物理化学および理論化学

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