UItrafast relaxation processes of Metal-to-Ligand Charge Transfer excited state in one-dimensional metal complex

Shinichiro Iwai, Toshihide Kamata, Kaoru Yamamoto, Toshiaki Ohta, Toshio Fukaya, Shigeo Murata

Research output: Contribution to journalArticlepeer-review

1 Citation (Scopus)

Abstract

We have investigated the optical response of Ni(dmg)2 thin film by pump-probe spectroscopy under excitation of the metal-to-ligand charge transfer(MLCT) absorption band. Almost the same photo-induced spectral change was observed as in the case of the resonant excitation to 1-D exciton absorption in Pt(dmg)2. It rises up within 200fs. This shows that the MLCT 'molecular ' excited state relaxes to 1-D intermolecular exciton state in such a short time.

Original languageEnglish
Pages (from-to)502-504
Number of pages3
JournalSpringer Series in Chemical Physics
Volume63
DOIs
Publication statusPublished - 1998
Externally publishedYes

ASJC Scopus subject areas

  • Physical and Theoretical Chemistry

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