Tunable two-dimensional electron system at the (110) surface of SnO2

J. Dai, E. Frantzeskakis, F. Fortuna, P. Lömker, R. Yukawa, M. Thees, S. Sengupta, P. Le Fèvre, F. Bertran, J. E. Rault, K. Horiba, M. Müller, H. Kumigashira, A. F. Santander-Syro

Research output: Contribution to journalArticlepeer-review

Abstract

We report the observation of a two-dimensional electron system (2DES) at the (110) surface of the transparent bulk insulator SnO2 and the tunability of its carrier density by means of temperature or Eu deposition. The 2DES is insensitive to surface reconstructions and, surprisingly, it survives even after exposure to ambient conditions- A n extraordinary fact recalling the well known catalytic properties SnO2. Our data show that surface oxygen vacancies are at the origin of such 2DES, providing key information about the long-debated origin of n-type conductivity in SnO2, at the basis of a wide range of applications. Furthermore, our study shows that the emergence of a 2DES in a given oxide depends on a delicate interplay between its crystal structure and the orbital character of its conduction band.

Original languageEnglish
Article number085121
JournalPhysical Review B
Volume101
Issue number8
DOIs
Publication statusPublished - 2020 Feb 15

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

Fingerprint Dive into the research topics of 'Tunable two-dimensional electron system at the (110) surface of SnO2'. Together they form a unique fingerprint.

Cite this