Transport dynamics of neutral excitons and trions in monolayer WS2

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38 Citations (Scopus)

Abstract

Understanding the spatial motion of excitons is of both fundamental interest and central importance for optoelectrical applications. Here, we have investigated the temperature (T) dependence of the transport dynamics of neutral excitons and charged excitons (trions) in atomically thin two-dimensional crystals of the transition-metal dichalcogenide WS2. The transport dynamics of neutral excitons can be divided into three temperature ranges, where the diffusion of neutral excitons is governed by thermal activation (≤∼75 K), ionized impurity scattering (∼75 K ≤ T ≤∼200 K), and LO phonon scattering (≥∼200 K). The trions have a diffusion length that is over 20 times longer than that of neutral excitons at very low temperatures (≤∼10 K), which may be related to theoretically predicted Pauli-blocking effects during the excitation process.

Original languageEnglish
Pages (from-to)9687-9694
Number of pages8
JournalACS Nano
Volume10
Issue number10
DOIs
Publication statusPublished - 2016 Oct 25

Keywords

  • WS
  • excitons
  • photoluminescence
  • temperature dependence
  • transport dynamics

ASJC Scopus subject areas

  • Materials Science(all)
  • Engineering(all)
  • Physics and Astronomy(all)

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