Three-electron interatomic coulombic decay from the inner-valence double-vacancy states in NeAr

T. Ouchi; K. Sakai; H. Fukuzawa; X. J. Liu; I. Higuchi; Y. Tamenori; K. Nagaya; H. Iwayama; M. Yao; D. Zhang; D. Ding; A. I. Kuleff; S. D. Stoychev; Ph V. Demekhin; N. Saito; K. Ueda

doi:10.1103/PhysRevLett.107.053401

Three-electron interatomic coulombic decay from the inner-valence double-vacancy states in NeAr

T. Ouchi, K. Sakai, H. Fukuzawa, X. J. Liu, I. Higuchi, Y. Tamenori, K. Nagaya, H. Iwayama, M. Yao, D. Zhang, D. Ding, A. I. Kuleff, S. D. Stoychev, Ph V. Demekhin, N. Saito, K. Ueda

Division of Measurements

Research output: Contribution to journal › Article › peer-review

16 Citations (Scopus)

Abstract

We have unambiguously identified interatomic Coulombic decay in NeAr from the inner-valence double-vacancy state Ne-Ar2⁺(3s^-2) to outer-valence triple-vacancy states Ne⁺(2p^-1)-Ar2 ⁺(3p^-2) by momentum-resolved electron-ion multicoincidence. This is the first observation of interatomic Coulombic decay where three electrons (3e) participate. The results suggest that this 3e interatomic Coulombic decay is significantly faster than other competing processes like fluorescence decay and charge transfer via curve crossing.

Original language	English
Article number	053401
Journal	Physical review letters
Volume	107
Issue number	5
DOIs	https://doi.org/10.1103/PhysRevLett.107.053401
Publication status	Published - 2011 Jul 26

ASJC Scopus subject areas

Physics and Astronomy(all)

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Ouchi, T., Sakai, K., Fukuzawa, H., Liu, X. J., Higuchi, I., Tamenori, Y., Nagaya, K., Iwayama, H., Yao, M., Zhang, D., Ding, D., Kuleff, A. I., Stoychev, S. D., Demekhin, P. V., Saito, N., & Ueda, K. (2011). Three-electron interatomic coulombic decay from the inner-valence double-vacancy states in NeAr. Physical review letters, 107(5), [053401]. https://doi.org/10.1103/PhysRevLett.107.053401

Three-electron interatomic coulombic decay from the inner-valence double-vacancy states in NeAr. / Ouchi, T.; Sakai, K.; Fukuzawa, H.; Liu, X. J.; Higuchi, I.; Tamenori, Y.; Nagaya, K.; Iwayama, H.; Yao, M.; Zhang, D.; Ding, D.; Kuleff, A. I.; Stoychev, S. D.; Demekhin, Ph V.; Saito, N.; Ueda, K.

In: Physical review letters, Vol. 107, No. 5, 053401, 26.07.2011.

Research output: Contribution to journal › Article › peer-review

Ouchi, T, Sakai, K, Fukuzawa, H, Liu, XJ, Higuchi, I, Tamenori, Y, Nagaya, K, Iwayama, H, Yao, M, Zhang, D, Ding, D, Kuleff, AI, Stoychev, SD, Demekhin, PV, Saito, N & Ueda, K 2011, 'Three-electron interatomic coulombic decay from the inner-valence double-vacancy states in NeAr', Physical review letters, vol. 107, no. 5, 053401. https://doi.org/10.1103/PhysRevLett.107.053401

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abstract = "We have unambiguously identified interatomic Coulombic decay in NeAr from the inner-valence double-vacancy state Ne-Ar2+(3s-2) to outer-valence triple-vacancy states Ne+(2p-1)-Ar2 +(3p-2) by momentum-resolved electron-ion multicoincidence. This is the first observation of interatomic Coulombic decay where three electrons (3e) participate. The results suggest that this 3e interatomic Coulombic decay is significantly faster than other competing processes like fluorescence decay and charge transfer via curve crossing.",

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AU - Ouchi, T.

AU - Sakai, K.

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AU - Liu, X. J.

AU - Higuchi, I.

AU - Tamenori, Y.

AU - Nagaya, K.

AU - Iwayama, H.

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AU - Zhang, D.

AU - Ding, D.

AU - Kuleff, A. I.

AU - Stoychev, S. D.

AU - Demekhin, Ph V.

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AU - Ueda, K.

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AB - We have unambiguously identified interatomic Coulombic decay in NeAr from the inner-valence double-vacancy state Ne-Ar2+(3s-2) to outer-valence triple-vacancy states Ne+(2p-1)-Ar2 +(3p-2) by momentum-resolved electron-ion multicoincidence. This is the first observation of interatomic Coulombic decay where three electrons (3e) participate. The results suggest that this 3e interatomic Coulombic decay is significantly faster than other competing processes like fluorescence decay and charge transfer via curve crossing.

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Three-electron interatomic coulombic decay from the inner-valence double-vacancy states in NeAr

Abstract

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