Thermally-stable high coercivity Ce-substituted hot-deformed magnets with 20% Nd reduction

Xin Tang, S. Y. Song, J. Li, H. Sepehri-Amin, T. Ohkubo, K. Hono

Research output: Contribution to journalArticlepeer-review

5 Citations (Scopus)

Abstract

We demonstrate a 20% Ce-substituted Nd-Fe-B hot-deformed magnet with a large coercivity (µ0Hc) of 1.69 T and a remanent magnetization of 1.32 T, which are comparable to those for Nd-Fe-B sintered magnets. The temperature coefficient of coercivity (β) of the Ce-substituted magnet was -0.593%/°C in the range of 27–127 °C, which is superior to that of a Nd-Fe-B sintered magnet (β = -0.669%/°C) with a comparable coercivity at room temperature. Furthermore, the coercivity and its thermal stability can be increased to µ0Hc =1.83 T and β = -0.51%/°C by applying the Nd80Cu20 eutectic grain boundary diffusion process to an optimized (Nd0.75Ce0.25)-Fe-B hot-deformed sample. A coercivity of 0.74 T was achieved at 150 °C in the Nd-Cu diffusion processed hot-deformed magnets, which is much higher than that of sintered magnets. Microstructure investigations and micromagnetic simulations indicate that the modification of grain boundary phase and formation of a Nd-rich shell near the grain boundaries of the developed (Nd,Ce)-Fe-B hot-deformed magnet is the cause of the improved coercivity at room temperature. Thus, in this work, we realize a microstructure-optimized low-cost (Nd0.8Ce0.2)-Fe-B hot-deformed magnet that can outperform Nd-Fe-B sintered magnets.

Original languageEnglish
Pages (from-to)8-15
Number of pages8
JournalActa Materialia
Volume190
DOIs
Publication statusPublished - 2020 May 15
Externally publishedYes

Keywords

  • Ce substitution
  • Coercivity
  • Hot-deformed magnet
  • Permanent magnet

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Ceramics and Composites
  • Polymers and Plastics
  • Metals and Alloys

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