Terahertz Faraday and Kerr rotation spectroscopy of Bi1-xSbx films in high magnetic fields up to 30 tesla

Xinwei Li, Katsumasa Yoshioka, Ming Xie, Timothy Ii G. Noe, Woojoo Lee, Nicolas Marquez Peraca, Weilu Gao, Toshio Hagiwara, Orjan S. Handegård, Li Wei Nien, Tadaaki Nagao, Masahiro Kitajima, Hiroyuki Nojiri, Chih Kang Shih, Allan H. MacDonald, Ikufumi Katayama, Jun Takeda, Gregory A. Fiete, Junichiro Kono

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2 Citations (Scopus)

Abstract

We report results of terahertz Faraday and Kerr rotation spectroscopy measurements on thin films of Bi1-xSbx, an alloy system that exhibits a semimetal-to-topological-insulator transition as the Sb composition x increases. By using a single-shot time-domain terahertz spectroscopy setup combined with a table-top pulsed minicoil magnet, we conducted measurements in magnetic fields up to 30 T, observing distinctly different behaviors between semimetallic (x<0.07) and topological insulator (x>0.07) samples. Faraday and Kerr rotation spectra for the semimetallic films showed a pronounced dip that blueshifted with the magnetic field, whereas spectra for the topological insulator films were positive and featureless, increasing in amplitude with increasing magnetic field and eventually saturating at high fields (>20 T). Ellipticity spectra for the semimetallic films showed resonances, whereas the topological insulator films showed no detectable ellipticity. To explain these observations, we developed a theoretical model based on realistic band parameters and the Kubo formula for calculating the optical conductivity of Landau-quantized charge carriers. Our calculations quantitatively reproduced all experimental features, establishing that the Faraday and Kerr signals in the semimetallic films predominantly arise from bulk hole cyclotron resonances while the signals in the topological insulator films represent combined effects of surface carriers originating from multiple electron and hole pockets. These results demonstrate that the use of high magnetic fields in terahertz magnetopolarimetry, combined with detailed electronic structure and conductivity calculations, allows us to unambiguously identify and quantitatively determine unique contributions from different species of carriers of topological and nontopological nature in Bi1-xSbx.

Original languageEnglish
Article number115145
JournalPhysical Review B
Volume100
Issue number11
DOIs
Publication statusPublished - 2019 Sep 19

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

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    Li, X., Yoshioka, K., Xie, M., Noe, T. I. G., Lee, W., Marquez Peraca, N., Gao, W., Hagiwara, T., Handegård, O. S., Nien, L. W., Nagao, T., Kitajima, M., Nojiri, H., Shih, C. K., MacDonald, A. H., Katayama, I., Takeda, J., Fiete, G. A., & Kono, J. (2019). Terahertz Faraday and Kerr rotation spectroscopy of Bi1-xSbx films in high magnetic fields up to 30 tesla. Physical Review B, 100(11), [115145]. https://doi.org/10.1103/PhysRevB.100.115145