多孔性硅基磷钼酸铵吸附剂对铯的固化性能

Translated title of the contribution: Solidification Characteristics of Porous AMP/SiO2 Towards Cs(Ⅰ)

Xiao Xia Zhang, Hao Wu, Yue Zhou Wei

Research output: Contribution to journalArticle

Abstract

AMP loaded silica adsorbents (AMP/SiO2) were synthesized by the rotary evaporation reducing pressure method and the crystallization method. A pressing/sintering method was used for the stable solidification of secondary solid wastes AMP-Cs/SiO2 which was produced from the separation of Cs from simulated high level liquid waste. The properties of the solidified products were investigated. Without allophane, the immobilization percentage of Cs (Ⅰ) decreases to 40% when the temperature is more than 1 000 ℃. When adding allophane, the stable Cs4Al4Si20O48 crystalline phase is recrystallized, the Cs immobilization percentage is more than 96% and the compressive strength is higher than 7 MPa. The leachability of Cs (Ⅰ) from the deionized water (DW) is about 3×10-5 g/(cm2•d) at 25 ℃.

Translated title of the contributionSolidification Characteristics of Porous AMP/SiO2 Towards Cs(Ⅰ)
Original languageChinese
Pages (from-to)51-57
Number of pages7
JournalHe-Huaxue yu Fangshe Huaxue/Journal of Nuclear and Radiochemistry
Volume42
Issue number1
DOIs
Publication statusPublished - 2020 Feb 20
Externally publishedYes

Keywords

  • AMP/SiO
  • Cs(Ⅰ)
  • CsAlSiO
  • Solidification

ASJC Scopus subject areas

  • Chemistry(all)
  • Nuclear and High Energy Physics

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