Revealing the ultrafast light-to-matter energy conversion before heat diffusion in a layered Dirac semimetal

Y. Ishida, H. Masuda, H. Sakai, S. Ishiwata, S. Shin

Research output: Contribution to journalArticlepeer-review

22 Citations (Scopus)

Abstract

There is still no general consensus on how one can describe the out-of-equilibrium phenomena in matter induced by an ultrashort light pulse. We investigate the pulse-induced dynamics in a layered Dirac semimetal SrMnBi2 by pump-and-probe photoemission spectroscopy. At 1 ps, the electronic recovery slowed upon increasing the pump power. Such a bottleneck-type slowing is expected in a two-temperature model (TTM) scheme, although opposite trends have been observed to date in graphite and in cuprates. Subsequently, an unconventional power-law cooling took place at ∼100 ps, indicating that spatial heat diffusion is still ill defined at ∼100ps. We identify that the successive dynamics before the emergence of heat diffusion is a canonical realization of a TTM scheme. Criteria for the applicability of the scheme is also provided.

Original languageEnglish
Article number100302
JournalPhysical Review B
Volume93
Issue number10
DOIs
Publication statusPublished - 2016 Mar 18
Externally publishedYes

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

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