Resonance-like enhancement in high-order above-threshold ionization of formic acid

C. Wang, Y. Tian, S. Luo, W. G. Roeterdink, Y. Yang, D. Ding, M. Okunishi, G. Prümper, K. Shimada, K. Ueda, R. Zhu

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20 Citations (Scopus)

Abstract

We have investigated the high-order above-threshold ionization (HATI) spectrum of formic acid by means of high-resolution electron spectroscopy using 800-nm femtosecond laser light. The resonance-like enhancement structures in the HATI spectrum are shown to be experimentally reproducible and three enhancement-suppression patterns are observed in different energy regimes with increasing laser intensity. We simulated these patterns successfully by computing the exact solution of time-dependent Schrödinger equation based on the simple hydrogen-like atom, subject to a time-dependent high-intensity laser pulse. The agreement between experiment and theory shows that "channel closing" effects play an important role in the observed resonance-like enhancements (RLEs). The existence of the RLEs for formic acid, which lacks any symmetry, shows that molecular symmetry does not affect the RLEs.

Original languageEnglish
Article number023405
JournalPhysical Review A - Atomic, Molecular, and Optical Physics
Volume90
Issue number2
DOIs
Publication statusPublished - 2014 Aug 6

ASJC Scopus subject areas

  • Atomic and Molecular Physics, and Optics

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