Radiocesium contamination in house dust within evacuation areas close to the Fukushima Daiichi nuclear power plant

Naohide Shinohara, Hiroko Yoshida-Ohuchi

Research output: Contribution to journalArticlepeer-review

12 Citations (Scopus)

Abstract

Outdoor decontamination efforts have been ongoing since the Fukushima Daiichi nuclear power plant (FDNPP) accident; however, little is known about indoor contamination. Therefore, house dust was sampled based on particle size in 21 wooden buildings (19 residential houses and 2 community centers) within the evacuation area close to the FDNPP, Fukushima Prefecture, Japan. Activities of radiocesium (137Cs) per gram of house dust increased with decreasing particle size (mean: 6.1 × 103, 2.6 × 103, 1.6 × 103, 7.5 × 102, 5.0 × 102, and 4.6 × 102 Bq/g for <4–20, 20–63, 63–180, 180–500, 500–1000, and 1000–2000 μm, respectively). The 137Cs concentrations in house dust were inversely related to the square of distance from the FDNPP for <4–1000 μm particles. From the results of the multiple linear regression analysis, distance from the FDNPP and direction from the FDNPP (northwest) were significantly related to the radioactivity of house dust. It was found that 19%, 33%, and 48% of 137Cs in house dust were extracted in water, 1 M HCl, and not extracted, respectively. Considering the bioaccessibility and assuming a 20 mg/day daily intake of house dust, the daily doses would be 7.2 Bq/day (mean) and 18 Bq/day (95th percent quantile). These results provide valuable insight into indoor radioactive Cs contamination in the area around the FDNPP and possible oral exposure to indoor radioactive Cs after returning home.

Original languageEnglish
Pages (from-to)107-114
Number of pages8
JournalEnvironment International
Volume114
DOIs
Publication statusPublished - 2018 May

Keywords

  • Extraction
  • Fukushima Daiichi nuclear power plant (FDNPP)
  • House dust
  • Indoor environment
  • Particle size
  • Radiocesium

ASJC Scopus subject areas

  • Environmental Science(all)

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