Quantum optimal control of unbounded molecular dynamics: Application to NaI predissociation

Kazuyuki Nakagami, Yukiyoshi Ohtsuki, Yuichi Fujimura

Research output: Contribution to journalArticlepeer-review

23 Citations (Scopus)

Abstract

For optimal control of unbounded molecular dynamics, an algorithm was developed to deal with a spatially delocalized final condition of pulse design equations by combining a target operating having the form of a quasiprojector with a wave packet splitting procedure. The resultant algorithm can be combined with the efficient iteration algorithms developed for solving the homogeneous type of pulse design equations. Thus, the obtained algorithm is a powerful tool for dealing with unbounded molecular dynamics such as photodissociation and bimolecular reactions.

Original languageEnglish
Pages (from-to)6429-6438
Number of pages10
JournalJournal of Chemical Physics
Volume117
Issue number14
DOIs
Publication statusPublished - 2002 Oct 8

ASJC Scopus subject areas

  • Physics and Astronomy(all)
  • Physical and Theoretical Chemistry

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