Quantum control of unidirectional rotations of a chiral molecular motor

M. Yamaki, K. Hoki, Yukiyoshi Ohtsuki, Hirohiko Kono, Y. Fujimura

Research output: Contribution to journalArticlepeer-review

11 Citations (Scopus)

Abstract

A quantum control method is presented for designing electric fields of laser pulses to drive a chiral molecular motor in desired, rotational directions. Intuitive or counter-intuitive rotational motion of a chiral motor, 2-chloro-5-methyl-cyclopenta-2,4-dienecarbaldehyde, was controlled by electric fields of ps-laser pulses with midinfrared central frequencies. The control mechanism is discussed by analyzing the time- and frequency-resolved spectrum of the electric fields of the laser pulses. Timing of laser pulses is the essential factor for controlling unidirectional motions.

Original languageEnglish
Pages (from-to)1900-1904
Number of pages5
JournalPhysical Chemistry Chemical Physics
Volume7
Issue number9
DOIs
Publication statusPublished - 2005 May 7

ASJC Scopus subject areas

  • Physics and Astronomy(all)
  • Physical and Theoretical Chemistry

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