Pressure-induced superconductivity in the iron-based ladder material BaFe 2 S 3

Hiroki Takahashi, Akira Sugimoto, Yusuke Nambu, Touru Yamauchi, Yasuyuki Hirata, Takateru Kawakami, Maxim Avdeev, Kazuyuki Matsubayashi, Fei Du, Chizuru Kawashima, Hideto Soeda, Satoshi Nakano, Yoshiya Uwatoko, Yutaka Ueda, Taku J. Sato, Kenya Ohgushi

Research output: Contribution to journalArticle

97 Citations (Scopus)

Abstract

All the iron-based superconductors identified so far share a square lattice composed of Fe atoms as a common feature, despite having different crystal structures. In copper-based materials, the superconducting phase emerges not only in square-lattice structures but also in ladder structures. Yet iron-based superconductors without a square-lattice motif have not been found, despite being actively sought out. Here, we report the discovery of pressure-induced superconductivity in the iron-based spin-ladder material BaFe 2 S 3, a Mott insulator with striped-type magnetic ordering below 1/4120 K. On the application of pressure this compound exhibits a metal-insulator transition at about 11 GPa, followed by the appearance of superconductivity below T c = 14 K, right after the onset of the metallic phase. Our findings indicate that iron-based ladder compounds represent promising material platforms, in particular for studying the fundamentals of iron-based superconductivity.

Original languageEnglish
Pages (from-to)1008-1012
Number of pages5
JournalNature Materials
Volume14
Issue number10
DOIs
Publication statusPublished - 2015 Oct 24

ASJC Scopus subject areas

  • Chemistry(all)
  • Materials Science(all)
  • Condensed Matter Physics
  • Mechanics of Materials
  • Mechanical Engineering

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    Takahashi, H., Sugimoto, A., Nambu, Y., Yamauchi, T., Hirata, Y., Kawakami, T., Avdeev, M., Matsubayashi, K., Du, F., Kawashima, C., Soeda, H., Nakano, S., Uwatoko, Y., Ueda, Y., Sato, T. J., & Ohgushi, K. (2015). Pressure-induced superconductivity in the iron-based ladder material BaFe 2 S 3. Nature Materials, 14(10), 1008-1012. https://doi.org/10.1038/nmat4351