Plasma catalysis for CO2 decomposition by using different dielectric materials

Ruixing Li, Qing Tang, Shu Yin, Tsugio Sato

Research output: Contribution to journalArticlepeer-review

50 Citations (Scopus)

Abstract

Despite a large of interest in the field of plasma assisted catalytic technology (PACT), very little has been reported on the catalysis of the different dielectric barriers for a dielectric barrier discharge (DBD) reaction. In the present study, Ca0.7Sr0.3TiO3 dielectric, that possesses both a high permittivity and a high dielectric strength, was prepared by a liquid phase sintering and used as a dielectric barrier to break CO2 in order to investigate the efficiency and characteristics of this ceramic on a plasma reaction in a DBD reactor. Its results were compared with commercial alumina and silica glass that possess lower permittivities, while were widely used in the previous studies. Not only the sinterability of the Ca0.7Sr0.3TiO3 dielectric was improved by the 0.5 wt.% Li2Si2O5 additive, but also both the mechanical and dielectric properties of the sintered bodies were increased significantly. This ceramic was successfully used as a barrier, and the CO2 conversion, which is proportional to permittivity, achieved 15.6%. It was much higher than with those using traditional alumina and silica glass barriers.

Original languageEnglish
Pages (from-to)617-622
Number of pages6
JournalFuel Processing Technology
Volume87
Issue number7
DOIs
Publication statusPublished - 2006 Jul
Externally publishedYes

Keywords

  • CaTiO
  • Carbon dioxide
  • Decomposition
  • Dielectric barrier discharge
  • Plasma
  • SrTiO

ASJC Scopus subject areas

  • Chemical Engineering(all)
  • Fuel Technology
  • Energy Engineering and Power Technology

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