Photon statistical effect on a three-level molecule in a strong laser field

Y. Nomura, Y. Ohtsuki, Y. Fujimura

Research output: Contribution to journalArticlepeer-review

1 Citation (Scopus)

Abstract

An expression for the time development of a three-level molecular system in a strong laser field that for the relevant absorption spectrum are derived taking into account the photon statistical effect. The field is assumed to be characterized by a coherent state in which the photons are distributed according to a Poisson distribution with mean photon number n. Model calculations of the time-dependent populations and the absorption spectra are carried out to demonstrate the photon statistical effects. The strong coherent field causes a beat localization of the population in a time domain, which does not appear in the number state field. The origin of the beat localization is clarified.

Original languageEnglish
Pages (from-to)365-373
Number of pages9
JournalChemical Physics
Volume131
Issue number2-3
DOIs
Publication statusPublished - 1989 Mar 15

ASJC Scopus subject areas

  • Physics and Astronomy(all)
  • Physical and Theoretical Chemistry

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