Multi hierarchical construction-induced superior capacitive performances of flexible electrodes for wearable energy storage

Liubing Dong, Gemeng Liang, Chengjun Xu, Wenbao Liu, Zheng Ze Pan, Enlou Zhou, Feiyu Kang, Quan Hong Yang

Research output: Contribution to journalArticlepeer-review

82 Citations (Scopus)

Abstract

A multi hierarchical construction is designed for flexible supercapacitor electrodes. Specifically, we chose activated carbon fiber cloth (ACFC) as flexible substrates, deposited polyaniline (PANI) on fiber surface first, then constructed continuous carbon nanotube (CNT) networks between fibers and finally deposited PANI on the CNT networks to obtain ACFC/PANI/CNT/PANI textile electrodes. Repeated deposition of PANI and application of ACFC substrate lead to high content of electrochemically active materials (i.e., PANI and activated carbon fiber); meanwhile, these active materials are located in different locations in the electrodes (fiber itself, fiber surface and the space between fibers), thus avoiding serious aggregation. The fabricated electrodes exhibit superior capacitive performances: areal capacitance, energy density and power density are 4039 mF cm−2, 131 μW h cm−2 and 11424 μW cm−2, respectively, remarkably higher than those of previously reported flexible supercapacitor electrodes; our electrodes also have good cycling stability and flexibility. Furthermore, high-performance thick electrodes (capacitance: 7804 mF cm−2; energy output: 214 μW h cm−2) and flexible fiber-like electrodes (capacitance: 805 mF cm−2; energy density: 23 μW h cm−2) are easily produced from our textile electrodes. This study offers a new direction for optimizing micro-structures and electrochemical properties of flexible electrodes in wearable energy storage devices.

Original languageEnglish
Pages (from-to)242-248
Number of pages7
JournalNano Energy
Volume34
DOIs
Publication statusPublished - 2017 Apr 1
Externally publishedYes

Keywords

  • Flexible supercapacitor
  • Multi hierarchical construction
  • Textile electrode
  • Wearable energy storage

ASJC Scopus subject areas

  • Renewable Energy, Sustainability and the Environment
  • Materials Science(all)
  • Electrical and Electronic Engineering

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