Magnetoelectric quasi-(0-3) nanocomposite heterostructures

Yanxi Li, Zhongchang Wang, Jianjun Yao, Tiannan Yang, Zhiguang Wang, Jia Mian Hu, Chunlin Chen, Rong Sun, Zhipeng Tian, Jiefang Li, Long Qing Chen, Dwight Viehland

    Research output: Contribution to journalArticlepeer-review

    80 Citations (Scopus)


    Magnetoelectric composite thin films hold substantial promise for applications in novel multifunctional devices. However, there are presently shortcomings for both the extensively studied bilayer epitaxial (2-2) and vertically architectured nanocomposite (1-3) film systems, restricting their applications. Here we design a novel growth strategy to fabricate an architectured nanocomposite heterostructure with magnetic quasiparticles (0) embedded in a ferroelectric film matrix (3) by alternately growing (2-2) and (1-3) layers within the film. The new heteroepitaxial films not only overcome the clamping effect from substrate, but also significantly suppress the leakage current paths through the ferromagnetic phase. We demonstrate, by focusing on switching characteristics of the piezoresponse, that the heterostructure shows magnetic field dependence of piezoelectricity due to the improved coupling enabled by good connectivity amongst the piezoelectric and magnetostrictive phases. This new architectured magnetoelectric heterostructures may open a new avenue for applications of magnetoelectric films in micro-devices.

    Original languageEnglish
    Article number6680
    JournalNature communications
    Publication statusPublished - 2015 Mar

    ASJC Scopus subject areas

    • Chemistry(all)
    • Biochemistry, Genetics and Molecular Biology(all)
    • Physics and Astronomy(all)


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