TY - JOUR
T1 - Local Density Fluctuation Governs the Divergence of Viscosity Underlying Elastic and Hydrodynamic Anomalies in a 2D Glass-Forming Liquid
AU - Shiba, Hayato
AU - Kawasaki, Takeshi
AU - Kim, Kang
N1 - Publisher Copyright:
© 2019 American Physical Society.
PY - 2019/12/23
Y1 - 2019/12/23
N2 - If a liquid is cooled rapidly to form a glass, its structural relaxation becomes retarded, producing a drastic increase in viscosity. In two dimensions, strong long-wavelength fluctuations persist, even at low temperature, making it difficult to evaluate the microscopic structural relaxation time. This Letter shows that, in a 2D glass-forming liquid, relative displacement between neighbor particles yields a relaxation time that grows in proportion to the viscosity. In addition to thermal elastic vibrations, hydrodynamic fluctuations are found to affect the long-wavelength dynamics, yielding a logarithmically diverging diffusivity in the long-time limit.
AB - If a liquid is cooled rapidly to form a glass, its structural relaxation becomes retarded, producing a drastic increase in viscosity. In two dimensions, strong long-wavelength fluctuations persist, even at low temperature, making it difficult to evaluate the microscopic structural relaxation time. This Letter shows that, in a 2D glass-forming liquid, relative displacement between neighbor particles yields a relaxation time that grows in proportion to the viscosity. In addition to thermal elastic vibrations, hydrodynamic fluctuations are found to affect the long-wavelength dynamics, yielding a logarithmically diverging diffusivity in the long-time limit.
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U2 - 10.1103/PhysRevLett.123.265501
DO - 10.1103/PhysRevLett.123.265501
M3 - Article
C2 - 31951456
AN - SCOPUS:85077319747
SN - 0031-9007
VL - 123
JO - Physical Review Letters
JF - Physical Review Letters
IS - 26
M1 - 265501
ER -