We have performed high-field and multi-frequency electron spin resonance (ESR) and magnetization measurements in magnetic fields up to about 53 T on single crystals of a delafossite triangular-lattice antiferromagnet CuCrO 2, which has been proposed to show an out-of-plane 120° spiral spin structure below about 24 K. We calculated ESR resonance modes and magnetization curves assuming an Ising-like Heisenberg Hamiltonian with a spiral spin structure by a mean-field theory. The experimental results can be well reproduced using the following parameters, the intralayer exchange constant J/k B=26.9 K, the easy-axis anisotropy D/k B=-0.47 K, and the in-plane g-factor g ab =2.0.
- High-field and multi-frequency ESR
- High-field magnetization
- Triangular lattice
ASJC Scopus subject areas
- Atomic and Molecular Physics, and Optics
- Materials Science(all)
- Condensed Matter Physics