TY - JOUR
T1 - Fluorine K-shell photoelectron angular distribution from CF4 molecules in the molecular frame
AU - Fukuzawa, H.
AU - Liu, X. J.
AU - Teranishi, T.
AU - Sakai, K.
AU - Prümper, G.
AU - Ueda, K.
AU - Morishita, Y.
AU - Saito, N.
AU - Stener, M.
AU - Decleva, P.
N1 - Funding Information:
The measurements were carried out with approval of JASRI and supported in part by Grants-in-Aid for Scientific Research from the Japan Society for the Promotion of Science (JSPS). The authors are grateful to the staff of SPring-8 for their help in the course of these studies. XJL gratefully acknowledges JSPS for financial support.
Copyright:
Copyright 2008 Elsevier B.V., All rights reserved.
PY - 2008/1/21
Y1 - 2008/1/21
N2 - Molecular-frame photoelectron angular distributions (MFPADs) for CF4 in the fluorine K-shell ionization region have been measured at three photon energies 705, 725 and 775 eV. The molecular axis was defined by the momenta of the F+ s(-) CF3+ ions detected in coincidence. The MFPADs were compared with ab initio calculations using the time dependent density functional theory. The results of a calculation assuming a localized F 1s core-hole agree better with the observed MFPADs than the results of a calculation using a delocalized core-hole, especially for 775 eV.
AB - Molecular-frame photoelectron angular distributions (MFPADs) for CF4 in the fluorine K-shell ionization region have been measured at three photon energies 705, 725 and 775 eV. The molecular axis was defined by the momenta of the F+ s(-) CF3+ ions detected in coincidence. The MFPADs were compared with ab initio calculations using the time dependent density functional theory. The results of a calculation assuming a localized F 1s core-hole agree better with the observed MFPADs than the results of a calculation using a delocalized core-hole, especially for 775 eV.
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U2 - 10.1016/j.cplett.2007.11.085
DO - 10.1016/j.cplett.2007.11.085
M3 - Article
AN - SCOPUS:38049049369
VL - 451
SP - 182
EP - 185
JO - Chemical Physics Letters
JF - Chemical Physics Letters
SN - 0009-2614
IS - 4-6
ER -