Fermi surface property and characteristic crystalline electric field effect in PrIr2Zn20

Masaki Matsushita, Jyunya Sakaguchi, Yuki Taga, Masahiro Ohya, Shingo Yoshiuchi, Hisashi Ota, Yusuke Hirose, Kentaro Enoki, Fuminori Honda, Kiyohiro Sugiyama, Masayuki Hagiwara, Koichi Kindo, Toshiki Tanaka, Yasunori Kubo, Tetsuya Takeuchi, Rikio Settai, Yoshichika Önuki

Research output: Contribution to journalArticle

16 Citations (Scopus)

Abstract

We measured the de Haas-van Alphen (dHvA) oscillations, electrical resistivity, magnetic susceptibility, magnetization, and specific heat of PrIr2Zn20, which has recently been suggested as a heavy-fermion superconductor. Several dHvA branches with small frequencies ranging from 0.33 × 106 to 8.00 × 106 Oe were detected in the dHvA experiment, which were well explained by the results of energy band calculations for LaIr2Zn20 using the lattice parameter of PrIr2Zn20. Moreover, the cyclotron effective mass is small, i.e., less than 1m0 (m0. rest mass of an electron). This means that 4f electrons are fully localized and do not contribute to the Fermi surface. Similar dHvA results were obtained for the reference compound LuIr2Zn20. Thus, superconductivity in PrIr2Zn20, which has been observed very recently below 0.05 K, is not due to heavy quasiparticles. In fact, the present superconductivity disappears at a magnetic field of 20 Oe. From the experimental results of magnetic susceptibility, magnetization, and specific heat, we estimated the 4f crystalline electric field (CEF) scheme of PrIr2Zn20: Γ3 (0 K)-Γ4 (separated from a non-Kramers Γ3 doublet by 36.0 K)-Γ1 (86.4 K)-Γ5 (103 K). On the basis of this CEF scheme, we discuss a broad Schottky peak in the magnetic specific heat at 0.4K and the metamagnetic-like anomaly of magnetization at Hm = 50 kOe for H || h100i.

Original languageEnglish
Article number074605
Journaljournal of the physical society of japan
Volume80
Issue number7
DOIs
Publication statusPublished - 2011 Jul 1
Externally publishedYes

Keywords

  • Crystalline electric field
  • Cyclotron effective mass
  • DHvA
  • Fermi surface
  • High-field magnetization
  • LuIrZn
  • Metamagnetic behavior
  • PrIrZn
  • Specific heat
  • Superconductivity

ASJC Scopus subject areas

  • Physics and Astronomy(all)

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  • Cite this

    Matsushita, M., Sakaguchi, J., Taga, Y., Ohya, M., Yoshiuchi, S., Ota, H., Hirose, Y., Enoki, K., Honda, F., Sugiyama, K., Hagiwara, M., Kindo, K., Tanaka, T., Kubo, Y., Takeuchi, T., Settai, R., & Önuki, Y. (2011). Fermi surface property and characteristic crystalline electric field effect in PrIr2Zn20. journal of the physical society of japan, 80(7), [074605]. https://doi.org/10.1143/JPSJ.80.074605