Femtosecond real-time probing of the ultrafast energy dissipation in the Hg(63P1)-CO van der Waals interaction

K. Ohmori, K. Amano, H. Chiba, M. Okunishi, Y. Sato

Research output: Contribution to journalArticle

5 Citations (Scopus)

Abstract

fs pump-probe experiment was performed on the B→a nonadiabatic dynamics in the Hg-CO vdW complex. Based on the observed wave packet propagation, the dynamics of the relevant nonadiabatic transition were identified. It was found that the transition occurs near the point where Hg and CO come nearest to each other on the B-state surface with a probability of 0.063 for a single approach of Hg and CO.

Original languageEnglish
Pages (from-to)461-464
Number of pages4
JournalJournal of Chemical Physics
Volume113
Issue number2
DOIs
Publication statusPublished - 2000 Jul 1

ASJC Scopus subject areas

  • Physics and Astronomy(all)
  • Physical and Theoretical Chemistry

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