TY - JOUR
T1 - Extended short-range ferromagnetic order with cluster-glass behavior in Dy2AuSi3
AU - Li, D. X.
AU - Nimori, S.
AU - Yamamura, T.
AU - Yubuta, K.
AU - Shirazaki, K.
AU - Zhao, X.
N1 - Copyright:
Copyright 2009 Elsevier B.V., All rights reserved.
PY - 2009/12/4
Y1 - 2009/12/4
N2 - We present the results of ac and dc susceptibilities, high-field magnetization, magnetic relaxation and electrical resistivity measurements for a ternary intermetallic compound Dy2AuSi3 with a hexagonal phase dominant crystal structure derived from the AlB2-type. Both the ac and dc susceptibilities show a field and frequency dependent peak around TC ∼ 12.5 K, while evident irreversible magnetism and long-time magnetic relaxation behavior can be observed below TC. These metastable magnetic properties suggest that an extended short-range ferromagnetic order occurs near TC, i.e. the formation of ferromagnetic cluster state. This is further confirmed by the magnetization and electrical resistivity measurements and by a dynamic analysis of the ac susceptibility data. According to the extended short-range ferromagnetic order model, ferromagnetic clusters in Dy2AuSi3 could exist with larger geometric dimensions, interact magnetically with each other and result in the observed cluster-glass behavior at low temperatures.
AB - We present the results of ac and dc susceptibilities, high-field magnetization, magnetic relaxation and electrical resistivity measurements for a ternary intermetallic compound Dy2AuSi3 with a hexagonal phase dominant crystal structure derived from the AlB2-type. Both the ac and dc susceptibilities show a field and frequency dependent peak around TC ∼ 12.5 K, while evident irreversible magnetism and long-time magnetic relaxation behavior can be observed below TC. These metastable magnetic properties suggest that an extended short-range ferromagnetic order occurs near TC, i.e. the formation of ferromagnetic cluster state. This is further confirmed by the magnetization and electrical resistivity measurements and by a dynamic analysis of the ac susceptibility data. According to the extended short-range ferromagnetic order model, ferromagnetic clusters in Dy2AuSi3 could exist with larger geometric dimensions, interact magnetically with each other and result in the observed cluster-glass behavior at low temperatures.
KW - Intermetallics
KW - Magnetic measurements
KW - X-ray diffraction
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U2 - 10.1016/j.jallcom.2008.11.034
DO - 10.1016/j.jallcom.2008.11.034
M3 - Article
AN - SCOPUS:70649083127
SN - 0925-8388
VL - 488
SP - 558
EP - 561
JO - Journal of Alloys and Compounds
JF - Journal of Alloys and Compounds
IS - 2
ER -