Examining the aerosol indirect effect over China using an SO₂ emission inventory

The relationship between SO₂ emissions and the effective particle radius of low-level water clouds (r_e) over China was investigated to determine anthropogenic effects on clouds. Sulfur dioxide emission values were obtained from a statistical inventory, and r_e origins were retrieved by satellite remote sensing on a 0.5° grid. Comparisons between annual mean SO₂ emissions and r_e showed generally decreasing r_e values, explained by the Twomey effect. The existence of the Twomey effect is supported by comparisons with simulated aerosol optical depths. Results further suggest that clouds over land show sensitivity to the Twomey effect as well as clouds over the ocean.