Competing spin modulations in the magnetically frustrated semimetal EuCuSb

Hidefumi Takahashi, Kai Aono, Yusuke Nambu, Ryoji Kiyanagi, Takuya Nomoto, Masato Sakano, Kyoko Ishizaka, Ryotaro Arita, Shintaro Ishiwata

Research output: Contribution to journalArticlepeer-review

Abstract

The competing magnetic ground states of the itinerant magnet EuCuSb, which has a hexagonal layered structure, were studied via magnetization, resistivity, and neutron-diffraction measurements on single-crystal samples. EuCuSb has a three-dimensional semimetallic band structure as confirmed by band calculation and angle-resolved photoelectron spectroscopy, consistent with the nearly isotropic metallic conductivity in the paramagnetic state. However, below the antiferromagnetic transition temperature of TN1 (8.5 K), the resistivity, especially along the hexagonal axis, increases significantly. This implies the emergence of anisotropic magnetic ordering coupled to the conducting electrons. Neutron-diffraction measurements show that the Eu spins, which order ferromagnetically within each layer, are collinearly modulated (up-up-down-down) along the hexagonal axis below TN1, followed by the partial emergence of helical spin modulation below TN2 (6 K). Based on the observation of anomalous magnetoresistance with hysteretic behavior, we discuss the competing nature of the ground state inherent in a frustrated Heisenberg-like spin system with a centrosymmetric structure.

Original languageEnglish
Article number174425
JournalPhysical Review B
Volume102
Issue number17
DOIs
Publication statusPublished - 2020 Nov 13

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

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