Coincidence momentum imaging of asymmetric Coulomb explosion of CO2 in phase-locked two-color intense laser fields

Tomoyuki Endo, Hikaru Fujise, Akitaka Matsuda, Mizuho Fushitani, Hirohiko Kono, Akiyoshi Hishikawa

Research output: Contribution to journalArticlepeer-review

6 Citations (Scopus)

Abstract

Coulomb explosion of CO2, CO2 → CO22+ + 2e- → CO+ + O+ + 2e-, in phase-locked two-color ultrashort intense laser fields (800 nm and 400 nm, ∼1014 W/cm2) has been investigated by coincidence momentum imaging. The momentum images of the O+ and CO+ fragments show asymmetric distributions along the laser polarization direction depending on the relative phase of the two-color laser fields. The fragment asymmetry becomes most prominent (∼4%) at the relative phases providing the largest asymmetry of the electric field amplitude, with the O+ fragments preferentially ejected to the stronger field side. The mechanism of the asymmetric bond breaking of the two equivalent C-O bonds is discussed in terms of the nuclear dynamics in CO22+.

Original languageEnglish
Pages (from-to)50-54
Number of pages5
JournalJournal of Electron Spectroscopy and Related Phenomena
Volume207
DOIs
Publication statusPublished - 2016 Feb 1

Keywords

  • CO
  • Coherent control
  • Coincidence momentum imaging
  • Coulomb explosion
  • Two-color intense laser field

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Radiation
  • Atomic and Molecular Physics, and Optics
  • Condensed Matter Physics
  • Spectroscopy
  • Physical and Theoretical Chemistry

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