Catalytic activity of carbon-supported iridium oxide for oxygen reduction reaction as a Pt-free catalyst in polymer electrolyte fuel cell

C. H. Chang; T. S. Yuen; Y. Nagao; H. Yugami

doi:10.1016/j.ssi.2011.06.015

Catalytic activity of carbon-supported iridium oxide for oxygen reduction reaction as a Pt-free catalyst in polymer electrolyte fuel cell

C. H. Chang, T. S. Yuen, Y. Nagao, H. Yugami

ENG - Mechanical Systems Engineering

Research output: Contribution to journal › Article › peer-review

15 Citations (Scopus)

Abstract

Iridium oxide supported on Vulcan XC-72 carbon black (IrO₂/C) as a cathode catalyst for polymer electrolyte fuel cell (PEFC) has been characterized by transmission electron microscopy (TEM) and X-ray diffraction (XRD) measurement. The IrO₂ particles were 8-160 nm in diameter. The oxygen electroreduction activity was studied by cyclic voltammetry (CV). It was found that IrO₂/C had high oxygen reduction reaction (ORR) activity. The performance of the membrane electrode assemble (MEA) was also tested in a single PEFC and showed that IrO₂/C catalyst would be potential candidates for use as cathode catalyst in PEFC.

Original language	English
Pages (from-to)	49-51
Number of pages	3
Journal	Solid State Ionics
Volume	197
Issue number	1
DOIs	https://doi.org/10.1016/j.ssi.2011.06.015
Publication status	Published - 2011 Aug 25

Keywords

Carbon-supported iridium oxide
Membrane electrode assemble
Oxygen reduction reaction
Polymer electrolyte fuel cell

ASJC Scopus subject areas

Chemistry(all)
Materials Science(all)
Condensed Matter Physics

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10.1016/j.ssi.2011.06.015

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title = "Catalytic activity of carbon-supported iridium oxide for oxygen reduction reaction as a Pt-free catalyst in polymer electrolyte fuel cell",

abstract = "Iridium oxide supported on Vulcan XC-72 carbon black (IrO2/C) as a cathode catalyst for polymer electrolyte fuel cell (PEFC) has been characterized by transmission electron microscopy (TEM) and X-ray diffraction (XRD) measurement. The IrO2 particles were 8-160 nm in diameter. The oxygen electroreduction activity was studied by cyclic voltammetry (CV). It was found that IrO2/C had high oxygen reduction reaction (ORR) activity. The performance of the membrane electrode assemble (MEA) was also tested in a single PEFC and showed that IrO2/C catalyst would be potential candidates for use as cathode catalyst in PEFC.",

keywords = "Carbon-supported iridium oxide, Membrane electrode assemble, Oxygen reduction reaction, Polymer electrolyte fuel cell",

author = "Chang, {C. H.} and Yuen, {T. S.} and Y. Nagao and H. Yugami",

note = "Funding Information: We thank the technical help from Dr. Kobayashi (Tohoku University) and Cabot Specialty Chemicals, Inc. (Tokyo, Japan) for the supply of Vulcan-XC72 carbon black. This study was supported by Improvement program of Research Environment for Young Researchers from Special Coordination Funds for Promoting Science and Technology (SCF) commissioned by the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan. This work was partly supported by the foundation of Hattori-Hokokai and the Japan Society for the Promotion of Science (JSPS) through the Funding Program for Next Generation World-Leading Researchers (NEXT Program), initiated by the Council for Science and Technology Policy (CSTP).",

year = "2011",

month = aug,

day = "25",

doi = "10.1016/j.ssi.2011.06.015",

language = "English",

volume = "197",

pages = "49--51",

journal = "Solid State Ionics",

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AU - Chang, C. H.

AU - Yuen, T. S.

AU - Nagao, Y.

AU - Yugami, H.

N1 - Funding Information: We thank the technical help from Dr. Kobayashi (Tohoku University) and Cabot Specialty Chemicals, Inc. (Tokyo, Japan) for the supply of Vulcan-XC72 carbon black. This study was supported by Improvement program of Research Environment for Young Researchers from Special Coordination Funds for Promoting Science and Technology (SCF) commissioned by the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan. This work was partly supported by the foundation of Hattori-Hokokai and the Japan Society for the Promotion of Science (JSPS) through the Funding Program for Next Generation World-Leading Researchers (NEXT Program), initiated by the Council for Science and Technology Policy (CSTP).

PY - 2011/8/25

Y1 - 2011/8/25

N2 - Iridium oxide supported on Vulcan XC-72 carbon black (IrO2/C) as a cathode catalyst for polymer electrolyte fuel cell (PEFC) has been characterized by transmission electron microscopy (TEM) and X-ray diffraction (XRD) measurement. The IrO2 particles were 8-160 nm in diameter. The oxygen electroreduction activity was studied by cyclic voltammetry (CV). It was found that IrO2/C had high oxygen reduction reaction (ORR) activity. The performance of the membrane electrode assemble (MEA) was also tested in a single PEFC and showed that IrO2/C catalyst would be potential candidates for use as cathode catalyst in PEFC.

AB - Iridium oxide supported on Vulcan XC-72 carbon black (IrO2/C) as a cathode catalyst for polymer electrolyte fuel cell (PEFC) has been characterized by transmission electron microscopy (TEM) and X-ray diffraction (XRD) measurement. The IrO2 particles were 8-160 nm in diameter. The oxygen electroreduction activity was studied by cyclic voltammetry (CV). It was found that IrO2/C had high oxygen reduction reaction (ORR) activity. The performance of the membrane electrode assemble (MEA) was also tested in a single PEFC and showed that IrO2/C catalyst would be potential candidates for use as cathode catalyst in PEFC.

KW - Carbon-supported iridium oxide

KW - Membrane electrode assemble

KW - Oxygen reduction reaction

KW - Polymer electrolyte fuel cell

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Catalytic activity of carbon-supported iridium oxide for oxygen reduction reaction as a Pt-free catalyst in polymer electrolyte fuel cell

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