Bulk 5f electronic states of the uranium monochalcogenide US as seen via soft x-ray photoemission

Y. Takeda, T. Okane, T. Ohkochi, Y. Saitoh, H. Yamagami, A. Fujimori, A. Ochiai

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5 Citations (Scopus)

Abstract

We have investigated the electronic states of the uranium monochalcogenide US, which is a typical ferromagnetic uranium compound, using soft x-ray photoemission spectroscopy (SX-PES). In early ultraviolet photoemission spectroscopy studies, two peak structures of the U5f states were observed and have been interpreted that one has an itinerant character around the Fermi level (EF) and the other located below EF has a character of localized U5f electrons. In this study, the intrinsic bulk valence-band spectrum of US was first deduced by estimating the contribution of surface states to the valence-band spectrum using core-level photoemission spectra. We conclude that the electronic structure of US can be basically described by the itinerant nature of the U5f electrons from comparison with theoretical valence-band spectra obtained by band-structure calculation in the local-density approximation.

Original languageEnglish
Article number161101
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume80
Issue number16
DOIs
Publication statusPublished - 2009 Oct 6

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

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