Application of a locally optimized control theory to pump-dump laser-driven chemical reactions

Y. Ohtsuki, Y. Yahata, H. Kono, Y. Fujimura

Research output: Contribution to journalArticlepeer-review

21 Citations (Scopus)

Abstract

A locally optimized control theory is developed. This theory is applied to pump-dump laser-driven chemical reactions via an electronically excited state. The results show that the theory can design the pulse shapes for chemical reactions with high quantum yields in strong laser intensity regimes in which perturbative treatments break down.

Original languageEnglish
Pages (from-to)627-631
Number of pages5
JournalChemical Physics Letters
Volume287
Issue number5-6
DOIs
Publication statusPublished - 1998 May 8

ASJC Scopus subject areas

  • Physics and Astronomy(all)
  • Physical and Theoretical Chemistry

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