TY - JOUR
T1 - Application of a locally optimized control theory to pump-dump laser-driven chemical reactions
AU - Ohtsuki, Y.
AU - Yahata, Y.
AU - Kono, Hirohiko
AU - Fujimura, Y.
N1 - Funding Information:
One of the authors (YF) gratefully acknowledges the Japan Society for the Promotion of Science for their support of the Japan–Canada joint research project `Control of Reaction Dynamics by Laser'. Thanks are also due to Professor A.D. Bandrauk and Dr. S. Chelkowski for their stimulating discussions. This work was partly supported by the Development of High-density Optical Pulse Generation and Advanced Material Control Techniques and also by a Grant-in-aid for Scientific Research (09740511).
PY - 1998/5/8
Y1 - 1998/5/8
N2 - A locally optimized control theory is developed. This theory is applied to pump-dump laser-driven chemical reactions via an electronically excited state. The results show that the theory can design the pulse shapes for chemical reactions with high quantum yields in strong laser intensity regimes in which perturbative treatments break down.
AB - A locally optimized control theory is developed. This theory is applied to pump-dump laser-driven chemical reactions via an electronically excited state. The results show that the theory can design the pulse shapes for chemical reactions with high quantum yields in strong laser intensity regimes in which perturbative treatments break down.
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U2 - 10.1016/S0009-2614(98)00224-3
DO - 10.1016/S0009-2614(98)00224-3
M3 - Article
AN - SCOPUS:0032495946
SN - 0009-2614
VL - 287
SP - 627
EP - 631
JO - Chemical Physics Letters
JF - Chemical Physics Letters
IS - 5-6
ER -