Abstract
Single-photon laser enabled Auger decay (spLEAD) is an electronic de-excitation process which was recently predicted and observed in Ne. We have investigated it using bichromatic phase-locked free electron laser radiation and extensive angle-resolved photoelectron measurements, supported by a detailed theoretical model. We first used separately the fundamental wavelength resonant with the Ne+ 2s-2p transition, 46.17 nm, and its second harmonic, 23.08 nm, then their phase-locked bichromatic combination. In the latter case the phase difference between the two wavelengths was scanned, and interference effects were observed, confirming that the spLEAD process was occurring. The detailed theoretical model we developed qualitatively predicts all observations: branching ratios between the final Auger states, their amplitudes of oscillation as a function of phase, the phase lag between the oscillations of different final states, and partial cancellation of the oscillations under certain conditions.
| Original language | English |
|---|---|
| Article number | 113036 |
| Journal | New Journal of Physics |
| Volume | 21 |
| Issue number | 11 |
| DOIs | |
| Publication status | Published - 2019 Nov 18 |
Keywords
- free-electron laser
- laser enabled Auger decay
- neon
ASJC Scopus subject areas
- Physics and Astronomy(all)
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A detailed investigation of single-photon laser enabled Auger decay in neon. / You, Daehyun; Ueda, Kiyoshi; Ruberti, Marco; Ishikawa, Kenichi L.; Carpeggiani, Paolo Antonio; Csizmadia, Tamás; Oldal, Lénárd Gulyás; N G, Harshitha; Sansone, Giuseppe; Maroju, Praveen Kumar; Kooser, Kuno; Callegari, Carlo; Fraia, Michele Di; Plekan, Oksana; Giannessi, Luca; Allaria, Enrico; Ninno, Giovanni De; Trov, Mauro; Badano, Laura; Diviacco, Bruno; Gauthier, David; Mirian, Najmeh; Penco, Giuseppe; Ribič, Primož Rebernik; Spampinati, Simone; Spezzani, Carlo; Mitri, Simone Di; Gaio, Giulio; Prince, Kevin C.
In: New Journal of Physics, Vol. 21, No. 11, 113036, 18.11.2019.Research output: Contribution to journal › Article › peer-review
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TY - JOUR
T1 - A detailed investigation of single-photon laser enabled Auger decay in neon
AU - You, Daehyun
AU - Ueda, Kiyoshi
AU - Ruberti, Marco
AU - Ishikawa, Kenichi L.
AU - Carpeggiani, Paolo Antonio
AU - Csizmadia, Tamás
AU - Oldal, Lénárd Gulyás
AU - N G, Harshitha
AU - Sansone, Giuseppe
AU - Maroju, Praveen Kumar
AU - Kooser, Kuno
AU - Callegari, Carlo
AU - Fraia, Michele Di
AU - Plekan, Oksana
AU - Giannessi, Luca
AU - Allaria, Enrico
AU - Ninno, Giovanni De
AU - Trov, Mauro
AU - Badano, Laura
AU - Diviacco, Bruno
AU - Gauthier, David
AU - Mirian, Najmeh
AU - Penco, Giuseppe
AU - Ribič, Primož Rebernik
AU - Spampinati, Simone
AU - Spezzani, Carlo
AU - Mitri, Simone Di
AU - Gaio, Giulio
AU - Prince, Kevin C.
N1 - Funding Information: DY wishes to thank support by JSPS KAKENHI Grant Number JP19J12870, and a Grant-in-Aid of Tohoku University Institute for Promoting Graduate Degree Programs, Division for Interdisciplinary Advanced Research and Education. This work was funded under the embedded CSE program of the ARCHERU.K. National Supercomputing Service (http://archer.ac.uk). This work was funded by EPSRC/DSTL MURI Grant EP/N018680/1. This work was supported in part by the x-ray Free Electron Laser Utilisation Research Project and the x-ray Free Electron Laser Priority Strategy Program of the Ministry of Education, Culture, Sports, Science, and Technology of Japan (MEXT) and theIMRAMprogram of Tohoku University, and the Dynamic Alliance for Open Innovation Bridging Human, Environment and Materials program. EVG, EIS andMMP acknowledge Foundation for the Advancement of Theoretical Physics and Mathematics BASIS.' KLI gratefully acknowledges support by the Cooperative Research Program of the Network Joint Research Center for Materials and Devices (Japan),' Grant-in-Aid for Scientific Research (Grant Nos. 16H03881 and 19H00869) from MEXT, the Center of Innovation Program from the Japan Science and Technology Agency, JST, CREST (Grant No. JPMJCR15N1), JST,MEXTQuantum Leap Flagship Program (MEXTQ-LEAP) Grant No. JPMXS0118067246, and Japan-Hungary Research Cooperative Program, JSPS and HAS.MMandTM acknowledge support by the Deutsche Forschungsgemeinschaft (DFG) under Grant No. SFB925/1.We acknowledge the support of the Alexander von Humboldt Foundation (Project Tirinto), the Italian Ministry of Research Project FIRB No.RBID08CRXK andNo. PRIN 2010 ERFKXL 006, the bilateral projectCNRJSPS Ultrafast science with extreme ultraviolet Free Electron Lasers, and funding from the European Union Horizon 2020 research and innovation program under the Marie Sklodowska-Curie Grant Agreement No. 641789 MEDEA(Molecular ElectronDynamics investigated by IntensE Fields and Attosecond Pulses).We thank Dr Robert Richter for a careful reading of the manuscript. Funding Information: Daehyun You Kiyoshi Ueda Marco Ruberti Kenichi L Ishikawa Paolo Antonio Carpeggiani Tam�s Csizmadia L�n�rd Guly�s Oldal Harshitha N G Giuseppe Sansone Praveen Kumar Maroju Kuno Kooser Carlo Callegari Michele Di Fraia Oksana Plekan Luca Giannessi Enrico Allaria Giovanni De Ninno Mauro Trov� Laura Badano Bruno Diviacco David Gauthier Najmeh Mirian Giuseppe Penco Primož Rebernik Ribič Simone Spampinati Carlo Spezzani Simone Di Mitri Giulio Gaio Kevin C Prince Daehyun You Kiyoshi Ueda Marco Ruberti Kenichi L Ishikawa Paolo Antonio Carpeggiani Tam�s Csizmadia L�n�rd Guly�s Oldal Harshitha N G Giuseppe Sansone Praveen Kumar Maroju Kuno Kooser Carlo Callegari Michele Di Fraia Oksana Plekan Luca Giannessi Enrico Allaria Giovanni De Ninno Mauro Trov� Laura Badano Bruno Diviacco David Gauthier Najmeh Mirian Giuseppe Penco Primož Rebernik Ribič Simone Spampinati Carlo Spezzani Simone Di Mitri Giulio Gaio Kevin C Prince Institute of Multidisciplinary Research for Advanced Materials, Tohoku University, Sendai 980-8577, Japan Department of Physics, Imperial College London, London SW7 2AZ, United Kingdom Department of Nuclear Engineering and Management, Graduate School of Engineering, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656, Japan Photon Science Center, Graduate School of Engineering, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656, Japan Research Institute for Photon Science and Laser Technology, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033, Japan Institut f�r Photonik, Technische Universit�t Wien, A-1040 Vienna, Austria ELI-ALPS, ELI-HU Non-Profit Ltd., Dugonics t�r 13, H-6720 Szeged, Hungary ELI-ALPS, Pint�r J�zsef utca, 6728 Szeged, Hungary Physikalisches Institut, Universit�t Freiburg, D-79106 Freiburg, Germany Department of Physics and Astronomy, University of Turku, Finland Elettra-Sincrotrone Trieste, I-34149 Basovizza, Trieste, Italy ENEA C.R. Frascati, I-00044 Frascati, Rome, Italy Laboratory of Quantum Optics, University of Nova Gorica, Nova Gorica 5001, Slovenia Centre for Translational Atomaterials, Swinburne University of Technology, Melbourne 3122, Australia Institute of Physics, University of Tartu, EST-50411 Tartu, Estonia Daehyun You, Kiyoshi Ueda, Marco Ruberti, Kenichi L Ishikawa, Paolo Antonio Carpeggiani, Tam�s Csizmadia, L�n�rd Guly�s Oldal, Harshitha N G, Giuseppe Sansone, Praveen Kumar Maroju, Kuno Kooser, Carlo Callegari, Michele Di Fraia, Oksana Plekan, Luca Giannessi, Enrico Allaria, Giovanni De Ninno, Mauro Trov�, Laura Badano, Bruno Diviacco, David Gauthier, Najmeh Mirian, Giuseppe Penco, Primož Rebernik Ribič, Simone Spampinati, Carlo Spezzani, Simone Di Mitri, Giulio Gaio and Kevin C Prince 2019-11-01 2019-11-18 13:41:58 cgi/release: Article released bin/incoming: New from .zip Original content from this work may be used under the terms of the Creative Commons Attribution 3.0 licence . Any further distribution of this work must maintain attribution to the author(s) and the title of the work, journal citation and DOI. Italian Ministry of Research PRIN 2010 ERFKXL 006 European Union Horizon 2020 Marie Sklodowska-Curie 641789 MEDEA JSPS KAKENHI JP19J12870 Cooperative Research Program of the \Network Joint Research Center for Materials and Devices (Japan)," 16H03881 17K05070 18H03891 19H00869 EPSRC/DSTL MURI EP/N018680/1 Center of Innovation Program from the Japan Science and Technology Agency, JST, CREST JPMJCR15N1 Deutsche Forschungsgemeinschaft https://doi.org/10.13039/501100001659 SFB925/1 Italian Ministry of Research Project FIRB RBID08CRXK yes Single-photon laser enabled Auger decay (spLEAD) is an electronic de-excitation process which was recently predicted and observed in Ne. We have investigated it using bichromatic phase-locked free electron laser radiation and extensive angle-resolved photoelectron measurements, supported by a detailed theoretical model. We first used separately the fundamental wavelength resonant with the Ne + 2 s –2 p transition, 46.17 nm, and its second harmonic, 23.08 nm, then their phase-locked bichromatic combination. In the latter case the phase difference between the two wavelengths was scanned, and interference effects were observed, confirming that the spLEAD process was occurring. The detailed theoretical model we developed qualitatively predicts all observations: branching ratios between the final Auger states, their amplitudes of oscillation as a function of phase, the phase lag between the oscillations of different final states, and partial cancellation of the oscillations under certain conditions. � 2019 The Author(s). Published by IOP Publishing Ltd on behalf of the Institute of Physics and Deutsche Physikalische Gesellschaft [1] Meitner L 1922 Z. Phys. 9 131–44 10.1007/BF01326962 Meitner L Z. Phys. 0044-3328 9 1922 131 144 [2] Auger P 1923 C. R. Hebd. Séances Acad. Sci. 177 169–71 Auger P C. R. Hebd. 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PY - 2019/11/18
Y1 - 2019/11/18
N2 - Single-photon laser enabled Auger decay (spLEAD) is an electronic de-excitation process which was recently predicted and observed in Ne. We have investigated it using bichromatic phase-locked free electron laser radiation and extensive angle-resolved photoelectron measurements, supported by a detailed theoretical model. We first used separately the fundamental wavelength resonant with the Ne+ 2s-2p transition, 46.17 nm, and its second harmonic, 23.08 nm, then their phase-locked bichromatic combination. In the latter case the phase difference between the two wavelengths was scanned, and interference effects were observed, confirming that the spLEAD process was occurring. The detailed theoretical model we developed qualitatively predicts all observations: branching ratios between the final Auger states, their amplitudes of oscillation as a function of phase, the phase lag between the oscillations of different final states, and partial cancellation of the oscillations under certain conditions.
AB - Single-photon laser enabled Auger decay (spLEAD) is an electronic de-excitation process which was recently predicted and observed in Ne. We have investigated it using bichromatic phase-locked free electron laser radiation and extensive angle-resolved photoelectron measurements, supported by a detailed theoretical model. We first used separately the fundamental wavelength resonant with the Ne+ 2s-2p transition, 46.17 nm, and its second harmonic, 23.08 nm, then their phase-locked bichromatic combination. In the latter case the phase difference between the two wavelengths was scanned, and interference effects were observed, confirming that the spLEAD process was occurring. The detailed theoretical model we developed qualitatively predicts all observations: branching ratios between the final Auger states, their amplitudes of oscillation as a function of phase, the phase lag between the oscillations of different final states, and partial cancellation of the oscillations under certain conditions.
KW - free-electron laser
KW - laser enabled Auger decay
KW - neon
UR - http://www.scopus.com/inward/record.url?scp=85071003521&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=85071003521&partnerID=8YFLogxK
U2 - 10.1088/1367-2630/ab520d
DO - 10.1088/1367-2630/ab520d
M3 - Article
AN - SCOPUS:85071003521
VL - 21
JO - New Journal of Physics
JF - New Journal of Physics
SN - 1367-2630
IS - 11
M1 - 113036
ER -